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Liu, H., Cheng, X., Chong, Y., Yuan, H., Huang, J.-Q., & Zhang, Q. (2021). Advanced electrode processing of lithium ion batteries: A review of powder technology in battery fabrication. Particuology, 57, 56-71. https://doi.org/https://doi.org/10.1016/j.partic.2020.12.003
Advanced electrode processing of lithium ion batteries: A review of powder technology in battery fabrication (Open Access)
He Liu a b, Xinbing Cheng c, Yan Chong c, Hong Yuan a b, Jia-Qi Huang a b *, Qiang Zhang c *
a School of Materials Science & Engineering, Beijing Institute of Technology, Beijing 100081, China
b Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, China
c Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China
10.1016/j.partic.2020.12.003
Volume 57, August 2021, Pages 56-71
Received 4 October 2020, Revised 16 December 2020, Accepted 17 December 2020, Available online 12 January 2021, Version of Record 23 February 2021.
E-mail: jqhuang@bit.edu.cn; zhang-qiang@mails.tsinghua.edu.cn

Highlights

• The basic principles of materials processing for lithium ion batteries

• The roles of slurry mixing and coating, electrode drying, and calendering

• Advancing powder technologies and related advanced energy materials



Abstract

Lithium ion batteries have achieved extensive applications in portable electronics and recently in electronic vehicles since its commercialization in 1990s. The vast applications of lithium ion batteries are not only derived from the innovation in electrochemistry based on emerging energy materials and chemical engineering science, but also the technological advances in the powder technologies for electrode processing and cell fabrication. Revealing the effects of powder technology on electrode microstructure evolution during electrode processing is with critical value to realize the superior electrochemical performance. This review presents the progress in understanding the basic principles of the materials processing technologies for electrodes in lithium ion batteries. The impacts of slurry mixing and coating, electrode drying, and calendering on the electrode characteristics and electrochemical performance are comprehensively analyzed. Conclusion and outlook are drawn to shed fresh lights on the further development of efficient lithium ion batteries by advancing powder technologies and related advanced energy materials.

Graphical abstract
Keywords
Lithium ion batteries; Composite electrode processing; Powder technology; Slurry coating and drying; Electrode calendering